Advances in Zeolite Catalysis for Conventional and Emerging Technologies: Zeolite Structure and Function
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Investigating the impact of the hydrophobic reaction environment of Lewis acid zeolites on catalytic activity for the epoxide ring opening with alcohols
Epoxides are important intermediates that are commonly ring opened using different nucleophiles to produce valuable bifunctional chemicals. Our recent work has shown that Sn-Beta is a highly active catalyst for epoxide ring opening provided that the substrates are small…
Adsorption and desorption of decalin, water and cyclohexanol in zeolites by in situ 2H MAS NMR and Computational Modeling
The adsorption and desorption of solvent (decalin and water) and reactant (cyclohexanol) on zeolites of MFI and FAU were investigated by in situ 2H magic angle spinning nuclear magnetic resonance (MAS NMR) and computational modeling…
Adsorption and desorption of decalin, water and cyclohexanol in zeolites by in situ 2H MAS NMR and Computational Modeling
The adsorption and desorption of solvent (decalin and water) and reactant (cyclohexanol) on zeolites of MFI and FAU were investigated by in situ 2H magic angle spinning nuclear magnetic resonance (MAS NMR) and computational modeling…
Impact of solvents on catalysis in micropores: Is the pore-half full or half-empty?
Catalytic reactions at solid-liquid interfaces involve complex networks of adsorption, surface reaction, and desorption processes, where each possesses a free energy of reaction and activation that contributes to measured rates and selectivities…