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(EDT)

Chemical Recycling & Upcycling of Polymers:

4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Credit
Overview
Division/Committee: [PMSE: Division of Polymeric Materials Science and Engineering]

Over 400 million tons of solid plastics are globally produced annually, but less than 9% of plastics is currently recycled. Traditional mechanical recycling of commodity polymers often present limitation due to undesirable degradation, oxidation, contamination, and altered molecular weight or composition. On the other hand, chemical recycling of polymers provides multiple paths for upcycled plastics. This symposium aims to feature recent advances in the fields of chemical recycling and upcycling of polymers. Specifically, the focus of the symposium includes synthesis of new polymers with closed-loop circularity, chemical upcycling paths for commodity plastics, synthetic paths for depolymerization and upcycling of polymers, dynamic polymers, and other polymer chemistry advances in chemical recycling.
Credits
0.00 CE
Organizers
Konstantinos Alexopoulos
Konstantinos Alexopoulos
The Pennsylvania State University
Mark Dadmun
Mark Dadmun
Univ of Tennessee
Brett Helms
Brett Helms
Staff Scientist
Lawrence Berkeley National Lab
Brian Long
Brian Long
Tomonori Saito
Tomonori Saito
Senior R&D staff
Oak Ridge National Laboratory
Hilal Ezgi Toraman
Hilal Ezgi Toraman
The Pennsylvania State University
Other
Poster - In-person
PMSE: Division of Polymeric Materials Science and Engineering
4178462 - Tailoring polythiophene nanocomposites with MnS/CoS nanoparticles for enhanced SERS detection of mercury ions in water | Poster Board #M33
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
The excessive emission of heavy metal ions from industrial processes poses a serious threat to both the environment and human health. This study presents a novel approach utilizing PTh-MnS/CoS NPs for the highly selective and sensitive detection of mercury ions in water…
Presenter
  • Temesgen Geremew Tefery
4183382 - Nitrene-facilitated dynamic crosslinking for compatibilization of HDPE/iPP blends with tunable thermomechnical properties | Poster Board #M35
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Polymer blends, which combine existing polymers, offer a cost-effective way to create new materials with enhanced properties. However, blending different polymers often results in phase separation and weak interfacial adhesion, leading to inferior performance…
Presenter
  • Roman Shrestha
Co-Author
  • Zhibin Guan
4185982 - Hydrophobic and UV-responsive crack-healable polymer to protect LiDAR sensor | Poster Board #M36
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
LiDAR sensors utilized in autonomous vehicles are exposed to external environments, making them susceptible to contamination…
Presenter
  • Jinho Kim
Co-Authors
  • Sunjong Lee
  • Kangtaek Lee, Yonsei University
4186475 - Synthesis of rigid polycyclic acetals from renewable feedstocks: A catalyst-free approach to bio-based platform chemicals | Poster Board #M25
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Monomers from biobased feedstocks continue to be developed for the production of high-performance thermosets. Cycloaliphatic or aromatic compounds are particularly desirable, as these structures are known to impart improved thermal and mechanical properties to resultant polymer networks…
Presenter
  • Jaclyn McLaughlin
Co-Author
  • Giuseppe Palmese
4186554 - Molecular design of capping agents for efficient chemical recycling of thermoplastic polyurethanes using blocked isocyanate chemistry | Poster Board #M26
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Polyurethanes are the 6th most used synthetic polymer with reported annual production of 26MMT in 2022. Thermoplastic polyurethanes (TPU) are a class of polyurethanes that distinguishes itself by its capacity to be melted and reshaped, unlike thermoset polyurethanes…
Presenter
  • Remsha Rafiq
Co-Authors
  • Jessica Gondak
  • Hannah Zucco
  • Stacey Ngo
  • Daylan Sheppard
  • Joeri Plusnin
  • Marie Anne Persoons
  • Glenn Cormack
  • Gotz Veser
4187199 - Withdrawn
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
4188314 - New compatibilization strategy for immiscible polymer blends | Poster Board #M34
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Phase separation between immiscible polymers presents a significant challenge in polymer blending and the recycling of mixed plastic waste. Immiscible polymer blends often undergo phase separation, leading to coarse phase morphologies like droplet-matrix structures…
Presenter
  • Leslie Liu
Co-Author
  • Zhibin Guan
4189525 - Withdrawn
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
4189589 - Base-catalyzed depolymerization of polyurethane foams to circular dicarbamate monomers | Poster Board #M27
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Polyurethanes (PUs) are the 6th most widely produced family of polymers and exist in an extensive array of formulations. PUs find application in foams for construction and comfort, elastomers for medical tubing and apparel, and coatings for waterproofing, flooring, and paint…
Presenter
  • Clarissa Westover, Arizona State University
Co-Author
  • Timothy Long, Virginia Tech
4189649 - Fully recyclable hemisiliconeelastomers with superior mechanical properties | Poster Board #M37
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Silicones are integral to a wide range of technologies, including elastomers, adhesives, cosmetics, coatings, and sealants. At the core of most silicone materials is polydimethylsiloxane (PDMS), characterized by its siloxane backbone (−(SiMe2−O)n−)…
Presenter
  • Shota Fujii
Co-Author
  • Thomas McCarthy
4191086 - Synthesis and depolymerization loop of ester-linked chemically recyclable polypropylene | Poster Board #M38
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
One of the most produced polymer materials, and the majority (~65%) of the thermoplastic polymer materials in use are polyolefins (POs). Based on 2012, only 16.2% of POs are recycled…
Presenter
  • Andrii Tiiara
Co-Authors
  • Bernadine Daichendt
  • Igor Luzinov
4191346 - Greener synthesis and shape-dependent degradation of Polynorbornenes | Poster Board #M39
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
As global plastic production continues to increase, plastic waste management has failed to keep up. This project aims to improve the efficiency of mechanical recycling of plastics by studying the relationship between polymer backbone stereochemistry and degradability…
Presenters
  • Greyson Karis-Sconyers
  • Britney Baez
Co-Author
  • Spencer Brucks
4191371 - Terminal-selective arylation of polyethylene | Poster Board #M40
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Polyethylene (PE) is a widely used commodity material for its low cost and versatile properties, commonly used for packaging films, insulation material, agricultural applications, etc…
Presenter
  • Julia Kim
Co-Authors
  • Molly McFadden, California Institute of Technology
  • John Hartwig
4191990 - Withdrawn
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
4192188 - Optimizing bottle-grade poly(ethylene terephthalate) characteristics in blends of bottle-grade and thermoform-grade poly(ethylene terephthalate) | Poster Board #M29
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Poly (ethylene terephthalate) (PET) is widely utilized in packaging applications in two primary forms: bottle grade (PET-B) and thermoform grade (PET-T)…
Presenter
  • Anurag Ganapathi
Co-Authors
  • Muhammad Rabnawaz, Ph.D., MICHIGAN STATE UNIVERSITY
  • Mohamed A Abdelwahab
4194121 - Withdrawn
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
4195723 - Withdrawn
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
4195965 - Withdrawn
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
4196064 - Withdrawn
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
4196090 - Selectively implosive chemical recycling of poly(ethylene terephthalate) | Poster Board #M41
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Poly(ethylene terephthalate) (PET) is a hydrophobic thermoplastic polyester with excellent thermomechanical, barrier, optical and chemical properties…
Presenter
  • Jared Kaczor
Co-Authors
  • Dhananjay Dileep, Iowa State University
  • Aadhi Subbiah
  • Michael Forrester
  • Eric Cochran, Iowa State University
4198046 - Impact of shear on dissolution kinetics of barrier layer from multilayer food packaging | Poster Board #M42
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Currently depolymerization or mechanical recycling of multilayer polymer structures does not produce quality materials due to recycling the materials simultaneously causing mixing of the polymers and reducing the properties of the resultant material…
Presenter
  • Marshall Smith
Co-Author
  • Edward Davis
4198532 - Incorporating reactive “Trojan horse” units for facile depolymerization of polyethylene terephthalate | Poster Board #M43
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Polyethylene terephthalate (PET) is a widely prevalent polyester used extensively in the packaging textile and beverage industries due to its thermomechanical ease in processing and superior chemical resistance…
Presenter
  • Aadhi Subbiah
Co-Authors
  • Dhananjay Dileep, Iowa State University
  • Jared Kaczor
  • Samuel Chambers
  • Aleksei Ananin
  • Shiva Karimi
  • Michael Forrester
  • Eric Cochran
4198558 - Ultrarobust, tough and highly stretchable self-healing UV curing elastomers based on induced entanglements with hyperbranched topological structures | Poster Board #M30
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Self-healable polymeric materials have found widespread applications, however the mechanical strength and healing efficiency of polymers has been proven extremely challenging…
Presenters
  • kejia ding
  • junheng zhang
4198785 - Unspooling polyethylene terephthalate (PET) at scale: tailored Terephthalates enable Lewis acid mediated depolymerization | Poster Board #M31
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
While PET is often touted as one of the most recycled plastics, current thermomechanical strategies rich in oxygen and moisture-rich environments at melt conditions lead to an unavoidable loss in molecular weight, necessitating chain extenders to recoup the loss in performance…
Presenter
  • Dhananjay Dileep, Iowa State University
Co-Authors
  • Aadhi Subbiah
  • Jared Kaczor
  • Samuel Chambers
  • Aleksei Ananin
  • Michael Forrester
  • Shiva Karimi
  • Gautham Pullela
  • George Kraus
  • Eric Cochran, Iowa State University
4198962 - Plastic’s Achilles Heel: Selectively Triggered chemical depolymerization of PET | Poster Board #M44
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
North American PET recycling rates, while on the rise, are still abysmally low. Bottle recycling rates reached 37.8% in 2022, while textile recycling remained stunted at 1%…
Presenter
  • Samuel Chambers
Co-Authors
  • Dhananjay Dileep, Iowa State University
  • Jared Kaczor
  • Aadhi Subbiah
  • Shiva Karimi
  • Aleksei Ananin
  • Michael Forrester
  • George Kraus
  • Eric Cochran, Iowa State University
4199018 - Terminal-selective amination of polyethylene | Poster Board #M45
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Polyethylene (PE) is a widely used polymer due to its low cost, durability, and versatility. However, its nonpolar backbone renders PE extremely hydrophobic and incompatible with polar surfaces…
Presenter
  • Pierre Lahaie-Boivin
Co-Authors
  • Molly McFadden, California Institute of Technology
  • John Hartwig
4199126 - Upcycling zero-valued poly(ethylene terephthalate): I. ammonolysis kinetics of model dimethyl terephthalate and catalytic effects of ethylene glycol | Poster Board #M47
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
Chemical upcycling of waste plastics can play an important role in developing greater circularity in the material flows associated with the plastics industries. In this study, a fundamental understanding of upcycling poly(ethylene terephthalate), PET, using ammonolysis is established…
Presenter
  • John Dorgan, Colorado School of Mines
Co-Author
  • Richard-Joseph Peterson
4200372 - Towards generation-invariant recyclable thermosets: three generations of deconstructable, recyclable polydicyclopentadiene with mild deconstruction strategies | Poster Board #M46
4:00 PM - 6:00 PM EDT
Wednesday, March 26, 2025Room: Pacific Ballroom Foyer (San Diego Marriott Marquis)
High-performance thermosets derive many of their desirable properties (e.g…
Presenter
  • Yasmeen AlFaraj
Co-Authors
  • Yuyan Wang
  • Edgar Mejia
  • Tyler Price
  • Suong Nguyen
  • Kwangwook Ko
  • Hayden Fowler
  • Samuel Leguizamon
  • Nancy Sottos
  • Jeremiah Johnson

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